Get Structural Glasses and Supercooled Liquids: Theory, PDF

By Peter G. Wolynes, Vassiliy Lubchenko

ISBN-10: 0470452234

ISBN-13: 9780470452233

ISBN-10: 1118202473

ISBN-13: 9781118202470

With contributions from 24 international specialists in diversified fields, and edited via world-recognized leaders in actual chemistry, chemical physics and biophysics, Structural Glasses and Supercooled beverages: thought, test, and Applications provides a latest, entire survey of glassy phenomena in lots of structures in response to firmly validated features of the underlying molecular motions as deduced through first precept theoretical calculations, or with direct/single-molecule experimental suggestions. A well-rounded view of a number of disordered structures the place cooperative phenomena, that are epitomized via supercooled beverages, ensue is provided.  those structures contain structural glasses and supercooled beverages, polymers, complicated drinks, protein conformational dynamics, and strongly interacting electron structures with quenched/self-generated ailment.

unique calculations and reasoned arguments heavily corresponding with experimental info are integrated, making the ebook obtainable to an informed non-expert reader. Content:
Chapter 1 Supercooled Liquid Dynamics: Advances and demanding situations (pages 1–30): Ranko Richert
Chapter 2 The Random First?Order Transition thought of Glasses: A serious evaluate (pages 31–113): Giulio Biroli and Jean?Philippe Bouchaud
Chapter three Dielectric Spectroscopy of Glassy Dynamics (pages 115–149): P. Lunkenheimer, M. Kohler, S. Kastner and A. Loidl
Chapter four Glasses and Replicas (pages 151–191): Marc Mezard and Giorgio Parisi
Chapter five Glassiness in Uniformly annoyed platforms (pages 193–221): M. Dzero, J. Schmalian and Peter G. Wolynes
Chapter 6 Random First?Order part Transition thought of the Structural Glass Transition (pages 223–236): T. R. Kirkpatrick and D. Thirumalai
Chapter 7 Fragile Glass Formers: proof for a brand new Paradigm, and a brand new Relation to powerful beverages (pages 237–278): C. Austen Angell
Chapter eight Dynamics within the Crossover zone of Supercooled beverages (pages 279–317): Biman Bagchi
Chapter nine Glassy Dynamics of Proteins (pages 319–339): Guo Chen, P. W. Fenimore and Hans Frauenfelder
Chapter 10 Theories of Structural Glass Dynamics: Mosaics, Jamming, and All That (pages 341–379): Vassiliy Lubchenko and Peter G. Wolynes

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With contributions from 24 worldwide specialists in different fields, and edited via world-recognized leaders in actual chemistry, chemical physics and biophysics, Structural Glasses and Supercooled beverages: thought, test, and purposes offers a latest, entire survey of glassy phenomena in lots of platforms according to firmly proven features of the underlying molecular motions as deduced by way of first precept theoretical calculations, or with direct/single-molecule experimental ideas.

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47] J. J¨ackle and R. Richert, Phys. Rev. E 77, 031201 (2008). [48] M. Maroncelli, J. Mol. Liq. 57, 1 (1993). [49] R. Richert, J. Chem. Phys. 113, 8404 (2000). [50] J. T. Fourkas, A. Benigno, and M. Berg, J. Chem. Phys. 99, 8552 (1993). [51] H. Wendt and R. Richert, J. Phys. Chem. A 102, 5775 (1998). -L. Horng, J. A. Gardecki, and M. Maroncelli, J. Phys. Chem. A 101, 1030 (1997). [53] G. B. Dutt and S. Raman, J. Chem. Phys. 114, 6702 (2001). [54] A. A. Ruth and B. Nickel, J. Phys. Chem. A 110, 3138 (2006).

For instance, the dependence of Tg on pressure p was found to display a wide range of sensitivities, with values for the pressure coefficient dTg /dp between 27 and 380K/GPa [73]. An alternative to reporting pressure effects on the dynamics is to describe the relaxation time in terms of an activation volume, VA , that is, the extra volume required by the activated state for structural relaxation to proceed [74, 75], τα (T, p) = τα (T, 0) exp p VA RT . 6) Expressions more reminiscent of the VFT form have also been used in order to account for a pressure–dependent effective activation volume [76, 77], τα (p) = τ0 exp Dp p p0 − p .

Ceram. Soc. 75, 1060 (1992). K. L. Ngaiand G. B. S. Department of Commerce, Springfield, VA, 1985. K. L. Ngai, E. Riande, and G. B. Wright, J. Non-Cryst. Solids 172–174, 1–1440 (1994). R. Richertand A. Blumen (eds), Disorder Effects on Relaxational Processes, Springer, Berlin, 1994. J. T. Fourkas, D. Kivelson, U. Mohanty, and K. A. Nelson (eds), Supercooled Liquids: Advances and Novel Applications, ACS Books, Washington, 1997. M. L. Williams, R. F. Landel, and J. D. Ferry, J. Am. Chem. Soc. 77, 3701 (1955).

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Structural Glasses and Supercooled Liquids: Theory, Experiment, and Applications by Peter G. Wolynes, Vassiliy Lubchenko


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